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Research advances on solvothermal conversion of levoglucosaninto value-added chemicals

2024 No. 02
253
178
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Authors:
TANG Guangchuan
HUANG Xin
QIN Hui
YU Feifan
LIU Tianlong
WEI Fu
RAN Jingyu
Unit:
Key Laboratory of Low-Grade Energy Utilization Technology and Systems of Ministry of Education,Chongqing University
Jiangsu Province Engineering Research Center of Fine Utilization of Carbon Resources,China University of Mining & Technology
Carbon Neutrality Institute,China University of Mining and Technology
Abstract:

Pyrolysis of lignocellulose is an efficient way to utilize biomass. The primary product of cellulose pyrolysis is levoglucosan(LGA), with a yield of up to 80%. Consequently, the high-value utilisation of LGA can be achieved through efficient conversion into other platform chemicals. The latest research progress on the pyrolysis of cellulose to LGA was presented, the influence of reactor types andreaction conditions on LGA yield were summarized, and biomass pretreatment could enhance the industrial scale production of LGA. ThenLGA conversion to levoglucosenone, glucose, and furan compounds under different conditions were concluded. It is found that Brønstedacid sites and in-situ removal of generated water during reaction improve levoglucosenone yield, with the maximum yield close to 60%,developing suitable catalysts and solvents can further improve levoglucosenone yield. Additionally, LGA can be effectively convertedto glucose by acid hydrolysis, attaining both yield and selectivity nearing 100%, and the catalyst with long-term stability, providing an indirect method for producing glucose from cellulose. Furthermore, the effects of catalysts and solvents on the formation of furanic compounds, acids and esters were summarized, indicating that these chemicals were formed via glucose as the intermediate.

Keywords:
biomass
solvothermal conversion
levoglucosan
levoglucosenone
glucose
furanic compounds
Citation format:
唐广川(1998—),男,重庆梁平人,硕士研究生。E-mail:tgc617@163.com
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Citation format:
TANG Guangchuan,HUANG Xin,QIN Hui,et al.Research advances on solvothermal conversion of levoglucosan into value-added chemicals[J].Clean Coal Technology,2024,30(2):143-152.

About Journal

  • Executive director

    China Coal Science and Industry Group Co., Ltd

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    Coal Science Research Institute Co., Ltd
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    Technology Research Center

  • Editor in Chief

    XIE Qiang

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    YU Chang
    SHI Yixiang
    ZHAO Yongchun
    DUAN Linbo
    CAO Jingpei
    ZENG Jie

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