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Research progress of coal fly ash for CO2 mineralization process

2024 No. 02
271
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Authors:
ZHANG Chujie
WANG Yugao
YAO Zhenchao
YANG Jiangfeng
Unit:
College of Chemical Engineering and Technology,Taiyuan University of Technology
Abstract:

CO2 mineralization is one of the key technologies to meet the challenge of global warming and other ecological problems causedby the massive emission of greenhouse gases such as CO2, which has become a major challenge to the survival of all mankind. The energyresource endowment pattern of " relatively coal-rich, oil-poor and gas-poor" has led to the fact that China′s main energy source is stilldominated by coal, which has a high CO2 emission intensity, and the industrial solid waste generated from the combustion of coal fly ashalso faces a huge problem of disposal. Compared with traditional mineralized raw materials, coal fly ash has received widespread attentiondue to its abundant reserves, easy accessibility and low transportation costs. Coal fly ash can achieve CO2 mineralization and sequestrationthrough direct and indirect mineralization, and reduce the environmental risks associated with the accumulation or disposal of coal fly ashwhile CO2 mineralization and sequestration is taking place. Under the goal of carbon peaking and carbon neutrality, the use of coal fly ashto mineralize and sequester CO2 is an efficient strategy with great potential to combat global warming. The current status of coal fly ashemissions and utilization in China were described. The research progress of direct and indirect coal fly ash mineralization was reviewed, theadvantages and disadvantages of different mineralization processes were compared and analyzed, the regulation mechanism of the processparameters on the efficiency of coal fly ash mineralization in the process of CO2 mineralization was clarified. In order to address the lackof mechanistic explanation of CO2 mineralization from coal fly ash, the mechanisms of gas-liquid diffusion and other mechanisms controlling the mineralization rate during the mineralization process were clarified through the introduction of the shrinking nucleus model and thesurface coverage model, which were commonly used to describe the CO2 mineralization reaction. Finally, the existing problems and futureresearch directions of the coal fly ash mineralization process were analyzed, aiming to provide a reference for the use of coal fly ash solidwaste to mineralize CO2.

Keywords:
CO2 mineralization
coal fly ash
direct mineralization
indirect mineralization
mineralization mechanism
Citation format:
张楚杰(2000—),男,湖南祁阳人,硕士研究生。E-mail:2861085377@qq.com
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Citation format:
ZHANG Chujie,WANG Yugao,YAO Zhenchao,et al.Research progress of coal fly ash for CO2 mineralization process[J].Clean Coal Technology,2024,30(2):300-315.

About Journal

  • Executive director

    China Coal Science and Industry Group Co., Ltd

  • Sponsored by

    Coal Science Research Institute Co., Ltd
    Coal Industry Clean Coal Engineering
    Technology Research Center

  • Editor in Chief

    XIE Qiang

  • Vice Editor-in-Chief

    YU Chang
    SHI Yixiang
    ZHAO Yongchun
    DUAN Linbo
    CAO Jingpei
    ZENG Jie

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    1006-6772

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    11-3676/TD

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