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Experiment of ammonia-coal co-firing in a drop tube furnace and thekinetic modeling of ammonia oxidation

2023 No. 09
441
193
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Authors:
YAN Weidong
QIN Shitai
YANG Kai
LI Guangbin
LI Ming
WANG Xuebin
TAN Houzhang
ZHANG Jiaye
Unit:
Beijing Guodian Electric Power Co.,Ltd.
National Energy Penglai Power Generation Co.,Ltd.
Sanhe Power Generation Co.,Ltd.
Hebei Coal-fired Power Station Pollution Prevention and Control Technology InnovationCenter
Yantai Longyuan Power Technology Co.,Ltd.
School of Energy and Power Engineering,Xi′an Jiaotong University
Abstract:

At present, the development of advanced carbon emission reduction technologies and the realization of the dual-carbon goalshave become the most urgent problems in the energy field. Carbon emissions from coal-fired power plants in China still account for a majorproportion. Ammonia, as a zero-carbon fuel, has significant advantages in heating value, synthesis, transportation and other aspects. Cofiring ammonia in coal-fired boilers is one of the important ways to achieve large-scale utilization, however, the control of nitrogen oxideemissions during large- scale co - firing will be a major challenge in the future. In this paper, the co - firing experiment of ammoniawith coal was carried out in a lab-scale furnace, and the effects of temperature (1 000-1 300 ℃ ), air/ fuel ratio(0.65-1.50), and cofiring ratio(0-30%) on nitrogen oxide emissions were discussed. The results show that the lower combustion temperature and air/ fuel ratiois essential to inhibit the conversion of ammonia to nitrogen oxides. Under the operating conditions of 1.5 air/ fuel ratio and 20% co-firingratio, the NOx emissions reach to 780×10-6 and 1 870×10-6 at 1 200 and 1 300 ℃ respectively. With the increase of ammonia ratio, theNOx emissionsincrease linearly, but the overall conversion of fuel nitrogen to NO decreases significantly. The calculations by detailed chemical reaction mechanisms (e.g. Glarborg 2018, Mendiara 2009, Konnov) show that the prediction results derived by Konnov mechanism are closer to the experimental results. The Konnov mechanism is further used to evaluate the influence of air/ fuel ratio,temperature and other variables on the NO emissions by ammonia combustion. The results show that the temperature and nitrogen oxideemission concentrations increase with exponential rate, while the total NOx emissions change abruptly when the air/ fuel ratio increasesfrom 1.0 to 1.1. A mixing factor is defined to study the effect of the mixing level of oxidant and ammonia on nitrogen oxide emissions, andit is found that prolonging the mixing distance of ammonia and oxidant can significantly reduce the intensity of nitrogen oxide emissions.

Keywords:
drop tube furnace
co-firing ammonia with coal
CO2 reduction
NOx emissions
Citation format:
闫卫东(1971—),男,辽宁义县人,高级工程师,硕士。E-mail:1944460140@qq.com
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Citation format:
YAN Weidong,QIN Shitai,YANG Kai,et al.Experiment of ammonia-coal co-firing in a drop tube furnace and the kinetic modeling of ammonia oxidation[J].Clean Coal Technology,2023,29(9):127-133.

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  • Executive director

    China Coal Science and Industry Group Co., Ltd

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    Coal Science Research Institute Co., Ltd
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    Technology Research Center

  • Editor in Chief

    XIE Qiang

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    YU Chang
    SHI Yixiang
    ZHAO Yongchun
    DUAN Linbo
    CAO Jingpei
    ZENG Jie

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