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Research process on ash chemistry of high-sodium coal during gasification

2023 No. 07
468
301
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Authors:
ZHANG Xianxian
BAI Jin
KONG Lingxue
LI Huaizhu
GUO Zhenxing
BAI Zongqing
LI Wen
Unit:
State Key Laboratory of Coal Conversion,Institute of Coal Chemistry of Chinese Academy of Sciences
University of Chinese Academy of Sciences
Abstract:

Coal gasification is a key technology to develop coal based bulk chemicals and clean fuels, and also an important way to achievethe goal of carbon neutrality. High sodium content and its volatilization of Zhundong coal during gasification lead to serious ash-releaseproblems. Therefore, it is of great significance to clarify the ash deposition and slagging mechanism and ash fluidity duringZhundong coal gasification for the clean and efficient utilization of high-sodium coal. Given this, the research progress on the ash chemis⁃try of high-sodium coal during gasification process was reviewed. The forms and content of sodium in coal were summarized. The migrationand transformation mechanisms of sodium in gasification and the ash deposition problem caused by sodium release on the heating surface ofthe gasifier were clarified. The ashing temperature is set at 500 ℃ because the sodium release in high sodium coal is mainly affected bythe gasification temperature. Low melting point sodium-containing minerals are easily generated during the gasification process, reducingthe ash melting temperature of high sodium coal ash. When the content of calcium and iron in high sodium coal is high, the formation oflow-temperature eutectic of anorthite and gehlenite in coal ash at high temperature, and the formation of low melting point spinel by Fe2+reacting with minerals in coal are important reasons for reducing coal ash melting temperature. Meanwhile, the atmosphere has a certain in⁃fluence on the minerals evolution of high-sodium coal during thermal conversion. The melting rate of high-sodium coal is fast,and the av⁃erage melting temperature is low, indicating that the ash has a strong fluidity. The Na2O can provide O2- and break the bridge oxygenbonds, causing the slag to depolymerize and reducing the viscosity value. The slag grid structure depolymerizes, the viscosity is reduced.The melting mechanism confirms the melting-dissolution mechanism. The precipitation of crystals in the slag during cooling has a crucialimpact on the viscosity. The introduction of Na2O reduces the crystallization temperature of slag and changes the crystal type. At the sametime, the viscosity activation energy and crystallization ability of the slag are reduced.

Keywords:
entrained flow gasification
high-sodium coal
ash deposition
ash fusion characteristics
viscosity-temperature characteristics
Citation format:
张显显(1991—),男,河南商丘人,博士研究生。E-mail:zxzzul@163.com
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Citation format:
ZHANG Xianxian,BAI Jin,KONG Lingxue,et al.Research process on ash chemistry of high-sodium coal during gasification[J].Clean Coal Technology,2023,29(7):110-124.

About Journal

  • Executive director

    China Coal Science and Industry Group Co., Ltd

  • Sponsored by

    Coal Science Research Institute Co., Ltd
    Coal Industry Clean Coal Engineering
    Technology Research Center

  • Editor in Chief

    XIE Qiang

  • Vice Editor-in-Chief

    YU Chang
    SHI Yixiang
    ZHAO Yongchun
    DUAN Linbo
    CAO Jingpei
    ZENG Jie

  • Publication Frequencies

    Monthly

  • ISSN

    1006-6772

  • CN

    11-3676/TD

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