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Research progress on the effect of iron on mineral transformation andmelting characteristics during coal gasification

2023 No. 07
517
283
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Authors:
SHEN Zhongjie
DONG Zizheng
LIANG Qinfeng
XU Jianliang
GUO Xiaolei
DAI Zhenghua
LIU Haifeng
Unit:
National Energy Coal Gasification Technology Research and Development Center,East China University of Science and Technology
Shanghai Engineering Research Center of Coal Gasification,East China University of Science and Technology
College of Chemical Engineering,Xinjiang University
Abstract:

Iron is an important element commonly found in coal minerals, and its occurrence parameters such as content and valence arethe key factors affecting the physical and chemical properties of coal gasification ash, such as mineral transformation, melting, crystalliza⁃tion, viscosity, rheology, etc. The type of coal used in gasifier and the change of operating conditions (atmosphere and temperature) af⁃fect the occurrence form of Fe, and the coal gasification ash containing iron shows different physical and chemical properties, which isof great significance to guide the smooth slagging of gasifier. Research progress on the occurrence form of iron in gasification ash, meltingproperties of Fe on coal gasification ash, crystallinity and viscosity-temperature properties during cooling process were reviewed. Fe mainlyexists in raw coal in the form of FeO, Fe2O3, FeS, and FeS2, and is converted into iron-containing aluminosilicates during coal gasifica⁃tion, which is significantly affected by gas compositions (CO/ CO2 / O2 / H2), chemical compositions and temperature. Due to Fe3+ has astrong polarity, it is difficult to react with other minerals, and the melting temperature of ash slag in oxidizing atmosphere is higher. WhileCO, H2 and other reducing gases have strong reducibility, Fe2O3 in ash slag is reduced to ferrous (Fe2+), its melting temperature is re⁃duced, but reduced to metallic iron (Fe), it has a high melting point characteristic, ash melting temperature increases. The effects of Fein coal gasification ash on the crystallization properties of molten liquid slag during the cooling process include the types of Fe-contai⁃ning crystals, crystallization temperature, crystallization conditions, crystal morphology and scale. Among them, the interaction of Fe andCa in aluminosilicate network structure is significantly affected by atmosphere, temperature and chemical composition. The main effect isthe interaction between the transformation of Fe/ Fe2+ / Fe3+ and calcium feldspar minerals, which affects the transformation of iron-contai⁃ning crystals and the precipitation of iron. The effect of Fe on the viscosity - temperature and viscosity - temperature characteristicsof coal gasification slag was discussed, including the variation of viscosity and the critical viscosity temperature, the different valencestates and contents of Fe were important parameters in the process of viscosity change and melt structure transformation. Finally, the effectof Fe on the physical and chemical properties of coal gasification ash was summarized. It is expected that the combined physical and chem⁃ical effects of iron elemental and ionic state ( Fe2+ / Fe3+ ) in complex atmosphere ( H2 / CO/ CO2 ) on mineral conversion, ash meltingand crystallization are the key to clarify the role of iron in coal gasification ash. It is necessary to establish a suitable prediction system forthe properties of iron coal gasification ash and slag to provide guidance for the operation of industrial gasifier.

Keywords:
coal gasification
ash and slag
iron
occurrence
phase transition
viscosity-temperature characteristics
Citation format:
沈中杰(1989—),男,浙江湖州人,特聘副研究员,博士。E-mail:zjshen@ecust.edu.cn
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Citation format:
SHEN Zhongjie,DONG Zizheng,LIANG Qinfeng,et al.Research progress on the effect of iron on mineral transformation and melting characteristics during coal gasification[J].Clean Coal Technology,2023,29(7):95-109.

About Journal

  • Executive director

    China Coal Science and Industry Group Co., Ltd

  • Sponsored by

    Coal Science Research Institute Co., Ltd
    Coal Industry Clean Coal Engineering
    Technology Research Center

  • Editor in Chief

    XIE Qiang

  • Vice Editor-in-Chief

    YU Chang
    SHI Yixiang
    ZHAO Yongchun
    DUAN Linbo
    CAO Jingpei
    ZENG Jie

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