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Investigation on the fragmentation behavior of coal and corresponding semicoke particles of different ranks at different residence time

2023 No. 06
344
119
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Authors:
QIAO Kai
ZHONG Shan
TANG Siyang
MA Kui
SONG Lei
YUE Hairong
LIANG Bin
Unit:
School of Chemical Engineering,Sichuan University
Institute of New Energy and Low-carbon Technology,Sichuan University
Abstract:

During the processes of coal combustion and gasification, the fragmentation of coal particle occurs throughout the whole reaction process. Coal particles fragment due to different reasons at different residence times, and the fragmentation behavior and particle size distribution variations caused by different mechanisms are also different. However, the fragmentation mechanisms and applicable models at different residence times are yet not clear. In order to investigate the fragmentation behavior of different coals and semi-cokes at different residence times, coals ofdifferent ranks including anthracite, bituminous coal, lignite and the corresponding semicokes were used as test samples for the high-temperature fragmentation experiments carried out in a horizontal-chamber furnace at 1 473 K under nitrogen atmosphere. In addition, a particle thermal stress model was developed with ANSYS finite element analysis software, and the fragmentation mechanism of different coals and their semicokes were analyzed based on the experimental and numerical simulation results. The simulation results show that the thermal stress induced primary fragmentation should occur in less than 2 s after heating for anthracite and different semicokes with low volatile matter content. As expected, the high-temperature fragmentation experiment also shows that these samples indeed only suffer thermal stress fragmentation in the initial 2 s. Bituminous coal and lignite continuously release volatiles during the residence time of 10 s, and the primary fragmentation occurs mainly due to the devolatilization. For the bituminous semicoke and lignite semicoke, numerous weak connections are produced during the pretreatment pyrolysis process, and obvious secondary fragmentation is observed in 6-10 s, and in the later period of the experiment, the fragmentation severity of the two semicoke samples is greater than that of the raw coal samples.

Keywords:
fragmentation
residence time
volatile matter
thermal stress
Citation format:
乔凯(1997—),男,甘肃庆阳人,硕士研究生。E-mail:qiaokai001@foxmail.com
[HT6H]通讯作者:[HTK][ZK(]钟山(1985—),男,四川内江人,副教授,博士。E-mail:zhongshan@scu.edu.cn
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Citation format:
QIAO Kai,ZHONG Shan,TANG Siyang,et al.Investigation on the fragmentation behavior of coal and corresponding semicoke particles of different ranks at different residence time[J].Clean Coal Technology,2023,29(6):173-179.

About Journal

  • Executive director

    China Coal Science and Industry Group Co., Ltd

  • Sponsored by

    Coal Science Research Institute Co., Ltd
    Coal Industry Clean Coal Engineering
    Technology Research Center

  • Editor in Chief

    XIE Qiang

  • Vice Editor-in-Chief

    YU Chang
    SHI Yixiang
    ZHAO Yongchun
    DUAN Linbo
    CAO Jingpei
    ZENG Jie

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    Monthly

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    1006-6772

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    11-3676/TD

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