Chinese Science Citation Database Core Library(CSCD)Source Journals
Chinese Core Journals
Chinese Core Science and Technology Journals
RCCSE China Authoritative Academic Journal(A+)
Dutch Digest and Citation Database (Scopus)

Analysis of migration characteristics of C/O/N elements in coal under preheated combustion reducing atmosphere

2022 No. 04
1011
388
OnlineView
Download
Authors:
ZHANG Yi
ZHU Jianguo
LYU Qinggang
ZHANG Xiaoyu
ZHANG Jiahang
PAN Fei
Unit:
Institute of Engineering Thermophysics,Chinese Academy of Sciences;University of Chinese Academy of Sciences
Abstract:

The deep control of the coal combustion process is the ultimate goal pursued by coal combustion researchers. Based on the gas conversion and the solid functional group conversion,the C/O/N element migration discipline of the fuel in the four reducing atmosphere regions was mainly analyzed and elaborated during the pulverized coal preheating combustion process. From the gas transformation analysis,it can be obtained that the carbon element in the whole process is mainly released in the form of CO and CO2,the oxygen element is mainly released with gaseous carbon oxide and nitrogen oxide,and the nitrogen element is mainly released in the form of N2 during the preheating stage. It is mainly released in the form of NO2 and NO during combustion stage,its nitrogen-containing form is related to the distance from the top of the combustion chamber. From the analysis of solid functional group transformation,it can be seen that the types of carbon-containing double bonds and nitrogen-containing functional groups on the surface of raw coal increase after preheating. In the three reducing regions of the combustion chamber,the carbon-containing double bonds on the fuel surface are consumed and generated for many times,the adsorbed oxygen on the surface is released and adsorbed for many times,and the types of nitrogen-containing functional groups also change. The preheated char and the solid sample at 400 mm generate the most carbon-containing double bonds and there is the regeneration of adsorbed oxygen,thus the samples generated at these two positions are the most active. The samples at 100 mm and 900 mm contain the most types of unstable N-containing functional groups,which makes the nitrogen in the sample easier to be released in the form of gas at these two locations. The experimental results can provide basic experimental data support for the depth control of NOx during coal combustion.

Keywords:
pulverized coal
preheating combustion
functional group transformation
occurrence form
NOx
reactivity
Citation format:
张毅(1996—),女,湖南娄底人,博士研究生。E-mail:zhangyi18@iet.cn
Chart:
Articles:
--
Citation format:
--

About Journal

  • Executive director

    China Coal Science and Industry Group Co., Ltd

  • Sponsored by

    Coal Science Research Institute Co., Ltd
    Coal Industry Clean Coal Engineering
    Technology Research Center

  • Editor in Chief

    XIE Qiang

  • Vice Editor-in-Chief

    YU Chang
    SHI Yixiang
    ZHAO Yongchun
    DUAN Linbo
    CAO Jingpei
    ZENG Jie

  • Publication Frequencies

    Monthly

  • ISSN

    1006-6772

  • CN

    11-3676/TD

Covered by

  • CSTPCD
  • RCCSE(A+)
  • AJ
  • EBSCO host
  • Ulrichsweb
  • JST
  • Scopus

Contact us

New Media

  • Meichuanmei
    Meichuanmei
  • Clean Coal Technology
    Clean Coal Technology
  • Online Journals
    Online Journals
Website Copyright © {year} Clean Coal Technology
京ICP备05086979号-19
地址:Coal Tower, Hepingli, Chaoyang District, Beijing, China.
邮编:100013
Tel:86-10-87986452 / 010-87986451
E-mail:jjmjs@263.net