Chinese Science Citation Database Core Library(CSCD)Source Journals
Chinese Core Journals
Chinese Core Science and Technology Journals
RCCSE China Authoritative Academic Journal(A+)
Dutch Digest and Citation Database (Scopus)

Effect of biomass ash on coal char gasification

2024 No. 02
283
100
OnlineView
Download
Authors:
DING Liang
ZHANG Xu
WEI Jiale
LI Wenyuan
LI Weipeng
WANG Zhiqing
FANG Yitian
Unit:
College of Chemistry and Chemical Engineering,Xi′an Shiyou University
State Key Laboratory of Coal Conversion,Institute of Coal Chemistry,Chinese Academy of Sciences
Abstract:

Biomass ash, rich in alkali and alkaline earth metals (AAEM), can be served as a natural catalyst in coal catalytic gasification.The promoting effect of biomass ash on coal gasification is a fundamental reason for the synergistic effect during co-gasification of biomassand coal. However, the AAEM in biomass ash may undergo deactivation during gasification, leading to the loss of catalytic activity. Theeffects of factors such as biomass ash type, content and temperature on coal char gasification through fixed-bed pyrolysis and gasificationexperiments were analyzed, combined with the analysis of XRD, Raman, XRF, and BET. The results indicate that the catalytic effect ofbiomass ash is related to the content and existing form of AAEM. The gasification reactivity of coal char increases with the increasing addition of wheat straw ash. However, when the addition of wheat straw ash reaches 40%, the reactivity of the coal char tends to changesmoothly. Wheat straw ash has an inhibitory effect on the gasification of coal char in the early stage of gasification reaction. As the carbon conversion increases, the catalytic effect of wheat straw ash decreases with the increasing temperature at the same conversion level. Inorder to inhibit the deactivation of potassium in wheat straw ash, eggshell was used as an additive to investigate the effects of mixing wheatstraw ash with eggshell on the gasification of coal char. The results indicate that the catalytic effect of wheat straw ash on the gasificationof coal char can be further enhanced by adding 25% wheat straw ash and 5% eggshell. The addition of wheat straw ash results in a largespecific surface area, an enriched pore structure, a more disordered carbon structure, a decrease in the gasification reaction activation energy and an increase in the gasification rate of the coal char. Random pore model is the most appropriate model to simulate the gasificationbehavior of coal char and the coal char with wheat straw ash. The findings provide a reference for the application of biomass ash incatalytic coal gasification.

Keywords:
biomass ash
catalytic coal gasification
alkali metal deactivation
calcium-based additive
gasification reaction kinetics
Citation format:
丁亮(1987—),男,山西长治人,讲师,博士。E-mail:dingliang6000@xsyu.edu.cn
Chart:
Articles:
--
Citation format:
DING Liang,ZHANG Xu,WEI Jiale,et al.Effect of biomass ash on coal char gasification[J].Clean Coal Technology,2024,30(2):72-83.

About Journal

  • Executive director

    China Coal Science and Industry Group Co., Ltd

  • Sponsored by

    Coal Science Research Institute Co., Ltd
    Coal Industry Clean Coal Engineering
    Technology Research Center

  • Editor in Chief

    XIE Qiang

  • Vice Editor-in-Chief

    YU Chang
    SHI Yixiang
    ZHAO Yongchun
    DUAN Linbo
    CAO Jingpei
    ZENG Jie

  • Publication Frequencies

    Monthly

  • ISSN

    1006-6772

  • CN

    11-3676/TD

Covered by

  • CSTPCD
  • RCCSE(A+)
  • AJ
  • EBSCO host
  • Ulrichsweb
  • JST
  • Scopus

Contact us

New Media

  • Meichuanmei
    Meichuanmei
  • Clean Coal Technology
    Clean Coal Technology
  • Online Journals
    Online Journals
Website Copyright © {year} Clean Coal Technology
京ICP备05086979号-19
地址:Coal Tower, Hepingli, Chaoyang District, Beijing, China.
邮编:100013
Tel:86-10-87986452 / 010-87986451
E-mail:jjmjs@263.net