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Hydrochlorination of acetylene performance over urea-modified Xinjiangcoal-based carbon supported copper catalyst

2024 No. 06
325
120
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Authors:
YANG Hailong
WANG Lu
YAN Haijun
SI Jianxin
WU Ronglan
LI Xiaofei
WANG Jide
GUAN Qingqing
SUN Hui
LIANG Changhai
Unit:
State Key Laboratory of Oil and Gas Fine Chemicals,Ministry of Education and Xinjiang Uyghur Autonomous Region,School ofChemical Engineering and Technology,Xinjiang University
State Key Laboratory of Chemistry and Utilizationof Carbon Based Energy Resources,Xinjiang University
Xinjiang Uygur Autonomous Region Product Quality Supervisionand Inspection Institute
State Key Laboratory of Fine Chemicals,Dalian University of Technology
Abstract:

Developing of environmental friendly,high-efficiency,stable and low-cost non-mercury catalyst is the key to PVC productionusing coal-route-based acetylene hydrochlorination. To improve the current problems of low catalytic activity and poor stability of copper(Cu)-based catalysts applied in the acetylene hydrochlorination reactions,a series of Cu/ Urea-CAC catalysts were prepared by urea modification strategies and the effects of the urea addition and Cu loading on the catalytic performances of catalysts for acetylene hydrochlorination were investigated. When the urea content is 15% and the Cu loading is 20%,the Cu/ Urea-CAC catalyst reveal the optimal catalyticperformance with the 92.6% C2H2 conversion and 98.2% vinyl chloride selectivity under the reaction conditions of 160 ℃ ,a C2 H2 gashourly space velocity of 120 h-1 and molar ratio of hydrogen chloride to acetylene is 1.25. Combination with the characterization results ofXPS,XRD,SEM,N2 adsorption and desorption,ICP -OES and TG techniques,it is suggested that the enhanced catalytic performanceis mainly related to the appropriate urea addition,which can effectively inhibit Cu species reduction and loss,and decrease the carbon deposition,thereby improving the catalytic performance activity of Cu-supported on Xinjiang coal-based carbon catalysts for acetylene hydrochlorination. The results will expand the application of Xinjiang coal-based carbon and provide theoretical support for the design,synthesisand catalysis of a new catalytic system for acetylene hydrochlorination.

Keywords:
scoal-based carbon
acetylene hydrochlorination
Cu catalysis
urea
modification
Citation format:
杨海龙(2000—),男,河南商丘人,硕士研究生。E-mail:1793221491@qq.com
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Citation format:
YANG Hailong, WANG Lu, YAN Haijun, et al. Hydrochlorination of acetylene performance over urea - modified Xinjiang coal-based carbon supported copper catalyst[J].Clean Coal Technology,2024,30(6):142-148.

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  • Executive director

    China Coal Science and Industry Group Co., Ltd

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    XIE Qiang

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    YU Chang
    SHI Yixiang
    ZHAO Yongchun
    DUAN Linbo
    CAO Jingpei
    ZENG Jie

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