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Research progress on the crystallization behavior of coal slag inentrained-flow gasifiers

2024 No. 06
724
167
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Authors:
LU Hao
BAI Jin
KONG Lingxue
GUO Zhenxing
LI Huaizhu
LI Wen
Unit:
State Key Laboratory of Coal Conversion,Institute of Coal Chemistry,Chinese Academy of Sciences
University of Chinese Academy of Sciences
Abstract:

Gasification is one of the important technologies to realize the transformation of coal from fuel to raw material and to promotethe clean and efficient utilization of coal. Entrained-flow gasification is currently the predominate gasification technology, and the stableoperation of gasifiers requires that the liquid slag must have good fluidity. The crystallization behavior of the slag can lead to decreasedflowability, resulting in abnormal shutdown of the gasifier, which is a major cause of abnormal shutdowns of gasifiers. The main crystallization characteristics were summarized and discussed that affected the fluidity of slag and the key to studying crystallization behavior: crystallization kinetics. Firstly, the methods of judging the crystallization mechanism based on crystallization behavior and selecting appropriate crystallization kinetics models were summarized. The principles and characteristics of different crystallization detection methodswere compared to obtain more accurate crystallization behavior data by selecting the appropriate crystallization behavior detection methodaccording to the research focus, facility characteristics and slag properties. Finally, the effects of chemical composition and operating conditions on crystallization behavior were summarized. Significant differences in the crystallization mechanisms between different crystals cause that the same chemical composition has different effects on the crystallization behavior of different crystals. When the chemical composition of the designated slag is within a specific phase region, the influence of chemical composition and operating conditionson crystallization behavior of the primary phase mineral becomes more regular, and the conclusions obtained can provide more accurate guidance for the regulation of crystallization behavior. Combining research results with phase diagrams or establishing simple and accessible predictive models can better guide the control of slag crystallization behavior. Currently, the study of crystallization behavior mainly relies on experimental methods. Future research could integrate phase-field simulation and molecular dynamics simulation, among other methods, to further explore the mechanisms of crystallization and examine the effects of factors such as temperature fields and flow fieldswithin gasifiers on crystallization characteristics.

Keywords:
entrained-flow gasification
slag flow behavior
mineral crystallization behavior
crystallization simulation
crystallization kinet ics
structure transformation
Citation format:
鲁浩(1996—),男,山东淄博人,博士研究生。E-mail:luhao@sxicc.ac.cn
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Citation format:
LU Hao,BAI Jin,KONG Lingxue,et al.Research progress on the crystallization behavior of coal slag in entrained-flow gasifiers[J].Clean Coal Technology,2024,30(6):47-67.

About Journal

  • Executive director

    China Coal Science and Industry Group Co., Ltd

  • Sponsored by

    Coal Science Research Institute Co., Ltd
    Coal Industry Clean Coal Engineering
    Technology Research Center

  • Editor in Chief

    XIE Qiang

  • Vice Editor-in-Chief

    YU Chang
    SHI Yixiang
    ZHAO Yongchun
    DUAN Linbo
    CAO Jingpei
    ZENG Jie

  • Publication Frequencies

    Monthly

  • ISSN

    1006-6772

  • CN

    11-3676/TD

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  • CSTPCD
  • RCCSE(A+)
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  • JST
  • Scopus

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