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Fabrication of porous carbon materials derived from high sulfur coal forenhanced lithium sulfur batteries performance

2024 No. 06
424
95
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Authors:
LIAO Mingyue
LEI Zhiping
JIA Tongxin
LI Yazhou
LI Zhanku
YAN Jingchong
SHUI Hengfu
YAN Honglei
REN Shibiao
WANG Zhicai
KANG Shigang
Unit:
Anhui Province Key Laboratory of Coal Clean Conversion and High Value-added Utilization,School of Chemistry &Chemical Engineering,Anhui University of Technology
Abstract:

Porous carbon materials with superior performance and low-cost have emerged as the preferred sulfur host materials in lithium-sulfur batteries, however, utilizing cheap raw materials to achieve large-scale preparation still faces great challenge. In this study, porous carbon materials were synthesized using abundant high sulfur coal as the feedstock and magnesium oxide and potassium hydroxide bothas templates and activators. The study delved into the investigation of structure-activity relationship of these materials when employed assulfur host materials in lithium sulfur batteries. It is observed that mesoporous (constituting 74%) are predominantly generated due to thetemplating action of MgO. KOH serves as an active agent primarily responsible for the formation of micropores ( constituting 72%).The combined use of MgO and KOH leads to the creation of carbon material, PCMgO+KOH, characterized by large specific surface area(1 616 m2 / g),high pore volume (1.02 m3 / g),and rich pore structure (54% mesoporous and 46% microporous). The results of electrochemical performance test show that the S@ PCMgO+KOH has good rate performance and excellent cycle stability. After 500 cycles of chargingang discharging at 1 C, it can still retain 553.2 mAh/ g, with a capacity retention rate of 65.5% and a decay rate of only 0.075% per cycle, demonstrating good rate performance and excellent cycling stability. The excellent electrochemical properties of PCMgO+KOH can be attributed mainly to its low ohmic resistance and charge transfer resistance, rapid polysulfide redox reaction kinetics, and exceptional capability in binding lithium polysulfide. This study provides an alternative route for the preparation of low-cost and high-performance host materials for lithium-sulfur batteries.

Keywords:
lithium-sulfur batteries
high sulfur coal
template agent
active agent
coal-based porous carbon
mesoporous structure
micro porous structure
Citation format:
廖明月(1999—),女,河南周口人,硕士研究生。E-mail:1204692922@qq.com
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Citation format:
LIAO Mingyue,LEI Zhiping,JIA Tongxin,et al.Fabrication of porous carbon materials derived from high sulfur coal for enhanced lithium sulfur batteries performance[J].Clean Coal Technology,2024,30(6):128-141.

About Journal

  • Executive director

    China Coal Science and Industry Group Co., Ltd

  • Sponsored by

    Coal Science Research Institute Co., Ltd
    Coal Industry Clean Coal Engineering
    Technology Research Center

  • Editor in Chief

    XIE Qiang

  • Vice Editor-in-Chief

    YU Chang
    SHI Yixiang
    ZHAO Yongchun
    DUAN Linbo
    CAO Jingpei
    ZENG Jie

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    11-3676/TD

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