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Heat transfer performance of sulfuric acid decomposition reactor inthermochemical sulfur iodine hydrogen production system

2024 No. 06
326
81
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Authors:
LI Mingyang
BIE Yiyan
HE Yong
WANG Bo
WANG Xiaoding
WANG Zhihua
Unit:
State Key Laboratory of Clean Energy Utilization,Zhejiang University
Dongfang Electric Co., Ltd.
Abstract:

The sulfuric acid decomposition reactor is an important equipment in the thermochemical sulfur iodine hydrogen production system, its heat transfer needs to match the hydrogen production capacity of the system. In order to study the effect of different structures ofsulfuric acid decomposition reactors on heat transfer, and to ensure that the heat transfer of the reactor meets the system requirements whilealso meeting the limitations of manufacturing processes. Through experiment, the reaction kinetics parameters of sulfuric acid decomposition reaction were calibrated and a reaction kinetics model was established. The reactor was simulated by gPROMS to obtain parameterssuch as pressure, temperature, flow rate, and component concentrations within the reactor. Results show that the total conversion rate cannot be improved by adjusting the length ratio of the preheating section and the reaction section or increasing the thermal conductivity of thepacked particles, while the total length of the reactor remains unchanged. Increasing the length of the preheating section in the reactor cansignificantly increase the total conversion rate. The key reason is that the length of the preheating section determines whether the temperature inside the reactor can reach the optimal temperature of 850 ℃ required for the SO3 decomposition reaction. Reducing the reactor diameter does not increase the total conversion rate, although reducing the diameter of the reactor is beneficial for heat transfer, due to the unchanged inlet flow rate, the fluid flow rate increases significantly, reducing the residence time of the reactants and significantly increasingthe reactor flow resistance. Using a sleeve annulus internal and external heating structure as the preheating section of the reactor can effectively improve the total conversion rate. When both internal and external heating are used, increasing the heat transfer area is beneficial forshortening the length of the preheating section. The length of the preheating section requires about 900 mm to achieve a reactor outlet temperature of 850 ℃ . A reactor structure design that meets the requirements has been found.

Keywords:
thermochemical H2 production
sulfur iodine cycle
sulfuric acid decomposition reactor
gPROMS
reactor structure
Citation format:
李明阳(1991—),男,四川成都人,工程师,硕士。E-mail:limy@dongfang.com
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Citation format:
LI Mingyang,BIE Yiyan,HE Yong,et al.Heat transfer performance of sulfuric acid decomposition reactor in thermochemicalsulfur iodine hydrogen production system[J].Clean Coal Technology,2024,30(6):180-188.

About Journal

  • Executive director

    China Coal Science and Industry Group Co., Ltd

  • Sponsored by

    Coal Science Research Institute Co., Ltd
    Coal Industry Clean Coal Engineering
    Technology Research Center

  • Editor in Chief

    XIE Qiang

  • Vice Editor-in-Chief

    YU Chang
    SHI Yixiang
    ZHAO Yongchun
    DUAN Linbo
    CAO Jingpei
    ZENG Jie

  • Publication Frequencies

    Monthly

  • ISSN

    1006-6772

  • CN

    11-3676/TD

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  • CSTPCD
  • RCCSE(A+)
  • AJ
  • EBSCO host
  • Ulrichsweb
  • JST
  • Scopus

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