Chinese Science Citation Database Core Library(CSCD)Source Journals
Chinese Core Journals
Chinese Core Science and Technology Journals
RCCSE China Authoritative Academic Journal(A+)
Dutch Digest and Citation Database (Scopus)

Effect of Mg modified CuZnAlY catalyst on the performance of CO2hydrogenation to methanol

2025 No. 03
109
81
OnlineView
Download
Authors:
WANG Lei
CUI Haitao
LI Guoqiang
LI Feng
LI Biao
LIU Gang
LI Lei
Unit:
College of Chemistry and Chemical Engineering,Taiyuan University of Technology
State Key Laboratory of CoalConversion,Institute of Coal Chemistry,Chinese Academy of Sciences
Abstract:

CO2 hydrogenation to methanol is an important way to achieve the goal of "double carbon". In this paper,CuZnAlY catalyst wasmodified by adding different contents of Mg,and its effect on the performance of CO2 hydrogenation to methanol was systematicallystudied. XRD,TPR,TPD and XPS were used to analyze the structure of the catalyst. The results showed that the addition of Mg built asuitable alkaline site,enhanced the CO2 adsorption capacity,improved the CO2 conversion and methanol selectivity. Among them,CZAYM2.5 composite catalyst has the highest space-time yield. Under the conditions of T=250 ℃,P=3.0 MPa,GHSV=4000 ml mlcat h,reaction gas H2:CO2=3:1 (molar ratio),the CO2 conversion,methanol selectivity and methanol space-time yield reached 18.95%,51.49% and 0.1549 g gcath,respectively. Meanwhile,stability tests were carried out for 720 h at improved pressure P=5.0 MPa. Theresults showed that:the CO2 conversion reached 22.00%,the selectivity of CH3OH was about 63.00%,and the methanol space-time yieldwas about 0.2100 g gcath. The catalyst showed good stability.

Keywords:
CO2 emissions
CO2 hydrogenation
Methanol
Composite catalyst
Mg modification
Citation format:
王雷(1997—),男,山西长治人,硕士研究生。E-mail:3194975948@qq.com
Chart:
--
Articles:
--
Citation format:
WANG Lei,CUI Haitao,LI Guoqiang,et al. Effect of Mg modified CuZnAlY catalyst on the performance of CO2hydrogenation to methanol[J].Clean Coal Technology,2025,31(3):72−82.

About Journal

  • Executive director

    China Coal Science and Industry Group Co., Ltd

  • Sponsored by

    Coal Science Research Institute Co., Ltd
    Coal Industry Clean Coal Engineering
    Technology Research Center

  • Editor in Chief

    XIE Qiang

  • Vice Editor-in-Chief

    YU Chang
    SHI Yixiang
    ZHAO Yongchun
    DUAN Linbo
    CAO Jingpei
    ZENG Jie

  • Publication Frequencies

    Monthly

  • ISSN

    1006-6772

  • CN

    11-3676/TD

Covered by

  • CSTPCD
  • RCCSE(A+)
  • AJ
  • EBSCO host
  • Ulrichsweb
  • JST
  • Scopus

Contact us

New Media

  • Meichuanmei
    Meichuanmei
  • Clean Coal Technology
    Clean Coal Technology
  • Online Journals
    Online Journals
Website Copyright © {year} Clean Coal Technology
京ICP备05086979号-19
地址:Coal Tower, Hepingli, Chaoyang District, Beijing, China.
邮编:100013
Tel:86-10-87986452 / 010-87986451
E-mail:jjmjs@263.net