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Technical status of carbon dioxide hydrogenation to methanol and researchprogress of catalysts

2025 No. 02
158
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Authors:
HE Nieyan
LI Xueqin
LIU Peng
CHEN Zhuo
ZHENG Binguo
LEI Tingzhou
Unit:
Changzhou Key Laboratory of Biomass Green,Safe,and High Value Utilization Technology,Institute of Urban and Rural Mines,Changzhou University
School of Management and Economics,North China University of Water Resources and Electric Power
School of civil engineering and architecture,Zhengzhou university of aeronautics
Abstract:

The combustion of fossil fuels emits a large amount of greenhouse gases.The study of carbon dioxide (CO2) emissionreduction and utilization has become a hot spot of worldwide concern and an urgent problem to be solved.The synthesis of methanol fromCO2 is an effective way to achieve large-scale low-carbon emission reduction and clean energy reproduction. However,there are still sometechnical problems in the process of CO2 conversion of high value-added products,such as unclear reaction active sites and high catalystcost. This paper takes the synthesis route of CO2 as raw material into high value-added chemicals as the starting point,introducing thetechnical route and development status of methanol synthesis from CO2 hydrogenation,and summarizes the factors affecting its selectivityin methanol synthesis process. It is found that catalyst is one of the important factors affecting the process of CO2 hydrogenation tomethanol and further compares the characteristics of different catalysts. In particular,copper-based catalysts have good catalytic activityfor the synthesis of high yield and high purity methanol. Finally,it analyzes the mechanism and existing problems of copper-basedcatalysts in methanol synthesis in detail, and the changes in the activity, selectivity and stability of the catalyst were analyzed from threeaspects:Active components,carriers and additives. In order to provide a theoretical reference for the preparation and screening of copper-based catalysts with high activity and low cost for CO2 hydrogenation to methanol,it also analyzes respectively the effects of activecomponents,supports and additives on the activity,selectivity and stability of the catalysts.

Keywords:
Carbon dioxide
clean utilization
catalyst
methanol
development status
Citation format:
何聂燕(1998—),女,广西藤县人,硕士研究生。E-mail:2438400586@qq.com
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Citation format:
HE Nieyan,LI Xueqin,LIU Peng,et al. Technical status of carbon dioxide hydrogenation to methanol and researchprogress of catalysts[J].Clean Coal Technology,2025,31(2):128−136.

About Journal

  • Executive director

    China Coal Science and Industry Group Co., Ltd

  • Sponsored by

    Coal Science Research Institute Co., Ltd
    Coal Industry Clean Coal Engineering
    Technology Research Center

  • Editor in Chief

    XIE Qiang

  • Vice Editor-in-Chief

    YU Chang
    SHI Yixiang
    ZHAO Yongchun
    DUAN Linbo
    CAO Jingpei
    ZENG Jie

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