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    加压循环流化床富氧燃烧中试研究

    Pilot-scale study on pressurized oxy-fuel combustion in circulating fluidized bed

    • 摘要: 二氧化碳捕集和封存技术(CCUS)是减少温室气体排放,实现全球环境可持续发展的有效技术手段。加压富氧燃烧技术是一种低成本CCUS技术。目前对于加压富氧燃烧研究大多处于理论建模、机理研究和小试试验阶段。中国科学院工程热物理研究所在MW级加压循环流化床富氧燃烧中试试验平台上进行了中试研究,顺利实现了加压富氧燃烧的稳定运行,工况运行中压力为0.30 MPa,功率为0.84 MW,尾部烟气中CO2浓度达到91%。此外,通过试验获得了中试尺度加压富氧燃烧运行模式,主要流程为:启动阶段-常压O2/N2燃烧阶段-常压富氧燃烧-加压富氧燃烧阶段,各个阶段切换平稳。

       

      Abstract: Carbon dioxide capture,utilization and storage(CCUS) is an effective technology to reduce greenhouse gas emissions and achieve sustainable development of the global environment. Pressurized oxy-fuel combustion technology is a low-cost CCUS technology.Circulating fluidized bed combustion technology( CFB) is one of the most commercialized clean coal combustion technologies. The pressurized CFB oxy-fuel combustion combines many advantages of pressurized oxy-fuel combustion and CFB combustion,which has a strong industrial application prospect. However,the complex structure,the switching of combustion conditions and the flue gas recirculation lead to the great challenges in the start-up,control and operation of the pressurized CFB oxy-fuel combustion system. At present,most of the researches on pressurized CFB oxy-fuel combustion are in the stage of theoretical modeling,mechanism research and bench-scale test. In order to further explore the start-up and operation methods of pressurized CFB oxy-fuel combustion,the pilot-scale experiment was carried out in a pilot test platform of MW pressurized CFB oxy-fuel combustion by Institute of Engineering Thermophysics,Chinese Academy of Sciences. The stable operation of pressurized oxy-fuel combustion was realized,and a pilot-scale pressurized oxy-fuel combustion operation mode and the variation curves of temperature,pressure,coal feed rate and air volume during start-up and operation were obtained.During the pressurized oxy-fuel combustion,the overall oxygen volume fraction reaches 29%,the operation pressure is 0. 30 MPa,the power is 0.84 MW,and the CO_2 volume fraction of the tail gas reaches 91%,which is benefit to the capture and compression purification of CO_2 product. The main process of the pilot-scale pressurized oxy-fuel combustion operation mode is as follows: start-up stage-atmospheric O_2/N_2 combustion stage-atmospheric oxy-fuel combustion-pressurized oxy-fuel combustion stage,and each stage switches stably.

       

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