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    MgO吸附剂捕集CO2的研究进展

    Research progress on MgO sorbents for CO_2 capture

    • 摘要: 煤大规模燃烧产生的CO2加剧了温室效应,CO2捕集、利用和储存(CCUS)是一种可实现燃煤电站大规模碳减排的关键技术。固体材料吸附CO2技术被认为是具有良好应用前景的碳捕集技术。在众多固体CO2吸附剂中,MgO因具有较高吸附容量、较低成本、较低再生能耗和广泛可用性被认为是理想的CO2吸附材料。本文综述了常规MgO的CO2吸附性能,针对MgO吸附CO2存在的问题,重点介绍了提高MgO吸附CO2性能的方法,主要包括优化结构和添加碱金属熔融盐等可行方法。最后综合分析了MgO吸附剂用于工业CO2捕集的优势及面临的挑战,并对今后的研究方向进行了展望。

       

      Abstract: Due to CO_2 produced by large-scale coal combustion aggravates the greenhouse effect,CO_2 capture,utilization and storage(CCUS) is a key technology to achieve large-scale carbon emission reduction at coal-fired power station.CO_2 adsorption by solid materials is considered as a promising carbon capture technology.Among many solid CO_2 adsorbents,MgO is considered as an ideal CO_2 adsorption material because of its high adsorption capacity,low cost,low regeneration energy consumption and wide availability.In this paper,the CO_2 adsorption performance of conventional MgO adsorbents was reviewed.According to the existing problems of CO_2 adsorption by MgO,the methods to improve the CO_2 adsorption performance by MgO were introduced,including the feasible methods such as optimizing the structure and adding alkali metal molten salt.Finally,the advantages and challenges of MgO adsorbents for industrial CO_2 capture were comprehensively analyzed.In addition,the research direction from the aspects of the fabrication strategy of MgO,large-scale molding of MgO pellets and CO_2 capture system design optimization using MgO in the future were prospected.

       

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